The maximum flow rate of a pump cannot be changed.
The 60psi or 100psi designation is not the pressure you will get out of the pump, but is the shut off pressure at which the pressure switch is set to turn the pump off. This can be altered slightly by adjusting the allen screw in the end of the pressure switch, BUT BE CAREFUL, this is usually for factory setting only.
SHURflo pumps currently used on Water Fed Pole applications are the 8000-441-138 (100psi, 4l/min) and 8000-946-138 (100psi, 5l/min) and are fitted with higher rated motors to suit the vigours of window cleaning.
If you have a 60psi pump it will probably be an old one originally designed for Agricultural Spraying applications with a lower rated motor designed for the intermittant duties of spraying.
See
www.williamsonpumps.co.uk for more details